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Disentangling Single- and Biexciton Dynamics with Photoelectron-Detected Two-Dimensional Electronic Spectroscopy
Action-detected two-dimensional (2D) spectroscopy resolves the time-dependent nonlinear optical response of a quantum system by recording incoherently detected observables such as fluorescence, photoelectrons, or photocurrents which reflect the system's excited-state population. Processes such as ex
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