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Quantitative Interleaved-Pulse Acquisition Extends the Range of Isotope-Ratio Measurements in ToF-SIMS
Isotope ratios underpin tracer studies of transport in oxides, battery materials, and biological systems, yet time-of-flight secondary ion mass spectrometry (ToF-SIMS) struggles to quantify ratios whose members differ in intensity by orders of magnitude: a primary-ion pulse long enough to count the
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