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Vibrational Sample-Based Quantum Diagonalization with Unitary-Cluster-Jastrow Ansätze on IBM QPUs
We extend sample-based quantum diagonalization (SQD) to anharmonic vibrational spectra and use it to benchmark how vibrational ansätze scale on present-day hardware under a direct one-hot encoding (up to 72 qubits). Five particle-conserving circuits are warm-started through vibrational coupled-clust
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