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Interfacial Coupling Reshapes Nonlinear Polarization in a Spin-Defect van der Waals Heterostructure
Van der Waals heterostructures offer a direct route to couple an optically active layer to a two-dimensional spin sensor, yet their coherent nonlinear response at interfaces remains poorly resolved. Here, we use polarization-resolved second harmonic-generation imaging to resolve four distinct region
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