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Hysteresis curves reveal the microscopic origin of cooperative CO2 adsorption in diamine-appended metal–organic frameworks
Diamine-appended metal-organic frameworks (MOFs) of the form Mg2(dobpdc)(diamine)2 adsorb CO2 in a cooperative fashion, exhibiting an abrupt change in CO2 occupancy with pressure or temperature. This change is accompanied by hysteresis. While hysteresis is suggestive of a first-order phase transitio
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