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Poly(vinylidene fluoride) under finite electric displacement fields: a removable $α\!\to\!δ$ reorientation barrier and a persistent first-order $δ\!\to\!β$ conformational change
The $α$, $δ$, and $β$ phases of PVDF are interconverted by electrical poling and mechanical drawing, yet the thermodynamics under a controlled electrical boundary condition has not been established from first principles. We evaluate the zero-temperature free energy at fixed electric displacement $D$
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