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Lone-Pair Stereoactivity Overrides Mass Scaling of Thermal Expansion and Heat Conduction in Non-vander Waals Layered Bismuth Oxychalcogenides
Heavier chalcogens are generally expected to soften isostructural semiconductor lattices, raising thermal expansion and lowering thermal conductivity. Layered bismuth oxychalcogenides, Bi2O2X (X = S, Se, Te), are mixed-anion crystals whose covalent slabs and ionic sheets are bound electrostatically
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