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Extreme Polarization of the Optical Gap and High-Energy Exciton Landscape in CrSBr
We reveal a strongly anisotropic excitonic landscape in monolayer and bulk-like CrSBr using optical absorption spectroscopy and $GW$-Bethe-Salpeter equation $\textit{ab initio}$ calculations. The direct absorptive determination of the lowest bright optical onsets i.e. $X_0^a$ and $X_0^b$ excitons fo
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