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Chemical Models of Nonheme Iron Monooxygenases; Reactive Intermediates and Catalytic Reactions
Nonheme에서의 산소화 효소 중간체인 Fe^(Ⅳ)=O종이 존재한다는 사실은 crystal구조로 인해 잘 알려져있다. 이 논문에서는 Nonheme 시스템에서 두가지 리간드를 이용한 Fe^(Ⅳ)=O종을 동위원소로 표지된 물실험(H₂^(18)O)을 통하여 oxygen exchange의 매카니즘을 규명하려고 한다. [Fe^(Ⅱ)(TMC)(OTf)₂]은 다양한 산화제와 반응하여 옅은 녹색의 반응 중간체인 [Fe^(Ⅳ)(O)(TMC)(NCCH₃)](OTf)₂종을 형성한다. 이 Fe^(Ⅳ)=O종을 thioanisole과 반응시키면 thioa
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