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Molecular Vibronic Complexity as a Quantum Resource for Optimal Control: Nonadiabatic Mixing Creates Protected Coherence Subspaces in Dissipative Environments

Palacino-González, Elisa
arXiv (All) · Papers
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chemical-physicsquantum-physics
In molecules, electronic coherence typically decays within a few hundred femtoseconds, a timescale usually attributed to the environment. We show that it is set to a large extent by which coherences are excited: the molecule can host coherences that the bath barely sees, and optimal control can find
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